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Abstract:
Lithium sulfur batteries (LSBs) with high energy density hold some promising applications in the wearable and flexible devices. However, it has been still challenging to develop a simple and feasible approach to prepare flexible LSB cathodes with both robust mechanical strength. Herein, flexible S@C-CNTs cathodes with controllable thicknesses are successfully fabricated via a facile blade-coating method. Due to the strong cohesion among CNTs bundles and the well-designed structure, the flexible S@C-CNTs cathodes are demonstrated to be with a combination of impressive mechanical strength and enhanced electrochemical performance. For the flexible S@C-CNTs cathodes with the sulfur mass loading of 4 mg cm−2, the areal capacity is close to 3.0 mA h cm−2, and the breaking stress is up to 5.59 MPa with 7.77% strain. Meanwhile, the pouch cell exhibits excellent cyclic stability at both flat/bent conditions. All demonstrate that the flexible S@C-CNTs cathodes may satisfy the demands of practical application. Moreover, this methodology is suitable for designing other flexible battery electrodes, such as flexible Si@C-CNTs anodes for lithium ion batteries, flexible P@C-CNTs anodes for sodium/potassium ion batteries, etc. © 2021 Elsevier Inc.
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Journal of Colloid and Interface Science
ISSN: 0021-9797
Year: 2021
Volume: 592
Page: 448-454
8 . 1 2 8
JCR@2020
ESI Discipline: CHEMISTRY;
ESI HC Threshold:32
CAS Journal Grade:3
Cited Count:
WoS CC Cited Count: 13
SCOPUS Cited Count: 28
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 9
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