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Author:

Xie, Chong (Xie, Chong.) | Shan, Hui (Shan, Hui.) | Song, Xuexia (Song, Xuexia.) | Chen, Liping (Chen, Liping.) | Wang, Jingjing (Wang, Jingjing.) | Shi, Jian-Wen (Shi, Jian-Wen.) | Hu, Junhua (Hu, Junhua.) | Zhang, Jiujun (Zhang, Jiujun.) | Li, Xifei (Li, Xifei.)

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EI SCIE PubMed Engineering Village

Abstract:

Lithium sulfur batteries (LSBs) with high energy density hold some promising applications in the wearable and flexible devices. However, it has been still challenging to develop a simple and feasible approach to prepare flexible LSB cathodes with both robust mechanical strength. Herein, flexible S@C-CNTs cathodes with controllable thicknesses are successfully fabricated via a facile blade-coating method. Due to the strong cohesion among CNTs bundles and the well-designed structure, the flexible S@C-CNTs cathodes are demonstrated to be with a combination of impressive mechanical strength and enhanced electrochemical performance. For the flexible S@C-CNTs cathodes with the sulfur mass loading of 4 mg cm−2, the areal capacity is close to 3.0 mA h cm−2, and the breaking stress is up to 5.59 MPa with 7.77% strain. Meanwhile, the pouch cell exhibits excellent cyclic stability at both flat/bent conditions. All demonstrate that the flexible S@C-CNTs cathodes may satisfy the demands of practical application. Moreover, this methodology is suitable for designing other flexible battery electrodes, such as flexible Si@C-CNTs anodes for lithium ion batteries, flexible P@C-CNTs anodes for sodium/potassium ion batteries, etc. © 2021 Elsevier Inc.

Keyword:

Anodes Cathodes Coatings Lithium-ion batteries Lithium sulfur batteries Stress analysis

Author Community:

  • [ 1 ] [Xie, Chong]Xi'an Key Laboratory of New Energy Materials and Devices, Institute of Advanced Electrochemical Energy, School of Materials Science and Engineering, Xi'an University of Technology, Xi'an; Shaanxi; 710048, China
  • [ 2 ] [Xie, Chong]Shaanxi International Joint Research Centre of Surface Technology for Energy Storage Materials, Xi'an; Shaanxi; 710048, China
  • [ 3 ] [Shan, Hui]Xi'an Key Laboratory of New Energy Materials and Devices, Institute of Advanced Electrochemical Energy, School of Materials Science and Engineering, Xi'an University of Technology, Xi'an; Shaanxi; 710048, China
  • [ 4 ] [Shan, Hui]Shaanxi International Joint Research Centre of Surface Technology for Energy Storage Materials, Xi'an; Shaanxi; 710048, China
  • [ 5 ] [Song, Xuexia]Xi'an Key Laboratory of New Energy Materials and Devices, Institute of Advanced Electrochemical Energy, School of Materials Science and Engineering, Xi'an University of Technology, Xi'an; Shaanxi; 710048, China
  • [ 6 ] [Song, Xuexia]Shaanxi International Joint Research Centre of Surface Technology for Energy Storage Materials, Xi'an; Shaanxi; 710048, China
  • [ 7 ] [Chen, Liping]Xi'an Key Laboratory of New Energy Materials and Devices, Institute of Advanced Electrochemical Energy, School of Materials Science and Engineering, Xi'an University of Technology, Xi'an; Shaanxi; 710048, China
  • [ 8 ] [Chen, Liping]Shaanxi International Joint Research Centre of Surface Technology for Energy Storage Materials, Xi'an; Shaanxi; 710048, China
  • [ 9 ] [Wang, Jingjing]Xi'an Key Laboratory of New Energy Materials and Devices, Institute of Advanced Electrochemical Energy, School of Materials Science and Engineering, Xi'an University of Technology, Xi'an; Shaanxi; 710048, China
  • [ 10 ] [Wang, Jingjing]Shaanxi International Joint Research Centre of Surface Technology for Energy Storage Materials, Xi'an; Shaanxi; 710048, China
  • [ 11 ] [Shi, Jian-Wen]State Key Laboratory of Electrical Insulation and Power Equipment, Center of Nanomaterials for Renewable Energy, School of Electrical Engineering, Xi'an Jiaotong University, Xi'an; 710049, China
  • [ 12 ] [Hu, Junhua]State Center for International Cooperation on Designer Low-carbon & Environmental Materials (CDLCEM), Zhengzhou University, 100 Kexue Avenue, Zhengzhou; 450001, China
  • [ 13 ] [Zhang, Jiujun]Xi'an Key Laboratory of New Energy Materials and Devices, Institute of Advanced Electrochemical Energy, School of Materials Science and Engineering, Xi'an University of Technology, Xi'an; Shaanxi; 710048, China
  • [ 14 ] [Zhang, Jiujun]Institute for Sustainable Energy/College of Science, Shanghai University, Shanghai; 200444, China
  • [ 15 ] [Li, Xifei]Xi'an Key Laboratory of New Energy Materials and Devices, Institute of Advanced Electrochemical Energy, School of Materials Science and Engineering, Xi'an University of Technology, Xi'an; Shaanxi; 710048, China
  • [ 16 ] [Li, Xifei]Shaanxi International Joint Research Centre of Surface Technology for Energy Storage Materials, Xi'an; Shaanxi; 710048, China

Reprint Author's Address:

  • [Shi, Jian-Wen]State Key Laboratory of Electrical Insulation and Power Equipment, Center of Nanomaterials for Renewable Energy, School of Electrical Engineering, Xi'an Jiaotong University, Xi'an; 710049, China;;

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Source :

Journal of Colloid and Interface Science

ISSN: 0021-9797

Year: 2021

Volume: 592

Page: 448-454

8 . 1 2 8

JCR@2020

ESI Discipline: CHEMISTRY;

ESI HC Threshold:32

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count: 13

SCOPUS Cited Count: 28

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 9

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