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Author:

Gu, Rui (Gu, Rui.) | Wang, Lei (Wang, Lei.) | Zhu, Huiping (Zhu, Huiping.) | Han, Shuangping (Han, Shuangping.) | Bai, Yurong (Bai, Yurong.) | Zhang, Xuewen (Zhang, Xuewen.) | Li, Bo (Li, Bo.) | Qin, Chengbing (Qin, Chengbing.) | Liu, Jie (Liu, Jie.) | Guo, Gang (Guo, Gang.) | Shan, Xiaoting (Shan, Xiaoting.) | Xiong, Guodong (Xiong, Guodong.) | Gao, Jiantou (Gao, Jiantou.) | He, Chaohui (He, Chaohui.) | Han, Zhengsheng (Han, Zhengsheng.) | Liu, Xinyu (Liu, Xinyu.) | Zhao, Fazhan (Zhao, Fazhan.)

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Abstract:

Solid-state quantum emitters play a critical role in the application of quantum information technology. Quantum emitters with high brightness at room temperature can be realized in hBN, and it has become a current research hotspot. However, much of the research up to now only produced quantum emitters at the edges and wrinkles of hBN, which tremendously limited the usage of the quantum emitters. In this work, heavy ions irradiation methods were employed to produce high-quality quantum emitters in the middle region of the hBN sample. The quantum emitter production engineering via heavy ions irradiation was systematically investigated. The dependence of irradiated ion type, energy, and fluence, as well as the thickness of the hBN flakes, on the production efficiency of the hBN quantum emitters were analyzed in detail. The characteristics of luminescence of quantum emitters, such as second-order correlation function g(2)(τ), stability, polarization, and saturation, were all compared with different irradiation conditions. In addition, based on the wavelength statistical results of quantum emitters in hBN, the transition energies of various intrinsic point defects in hBN were studied through first-principles calculations to reveal the originations of luminescence. The calculation results indicated that the VN, VB, and Bi point defects were possible candidates of the quantum emitter centers. Overall, in this study, according to experimental characterizations, heavy ion irradiation should be an efficient method to produce stable, ultrabright, highly linearly polarized quantum emitters in hBN flakes. © 2021 American Chemical Society.

Keyword:

Calculations Heavy ions Ion bombardment Luminescence Point defects Polarization Quantum efficiency Quantum optics

Author Community:

  • [ 1 ] [Gu, Rui]The University of Chinese Academy of Sciences, Beijing; 100029, China
  • [ 2 ] [Gu, Rui]The Key Laboratory of Science and Technology on Silicon Devices, Institute of Microelectronics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 3 ] [Wang, Lei]The Key Laboratory of Science and Technology on Silicon Devices, Institute of Microelectronics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 4 ] [Zhu, Huiping]The Key Laboratory of Science and Technology on Silicon Devices, Institute of Microelectronics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 5 ] [Han, Shuangping]State Key Laboratory of Quantum Optics and Quantum Optics Devices, Institute of Laser Spectroscopy, Shanxi University, Shanxi Province, Taiyuan; 030006, China
  • [ 6 ] [Han, Shuangping]Collaborative Innovation Center of Extreme Optics, Shanxi University, Shanxi Province, Taiyuan; 030006, China
  • [ 7 ] [Bai, Yurong]School of Nuclear Science and Technology, Xi'An JiaoTong University, Shaanxi Province, Xi'an; 710049, China
  • [ 8 ] [Zhang, Xuewen]The Key Laboratory of Science and Technology on Silicon Devices, Institute of Microelectronics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 9 ] [Li, Bo]The Key Laboratory of Science and Technology on Silicon Devices, Institute of Microelectronics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 10 ] [Qin, Chengbing]State Key Laboratory of Quantum Optics and Quantum Optics Devices, Institute of Laser Spectroscopy, Shanxi University, Shanxi Province, Taiyuan; 030006, China
  • [ 11 ] [Qin, Chengbing]Collaborative Innovation Center of Extreme Optics, Shanxi University, Shanxi Province, Taiyuan; 030006, China
  • [ 12 ] [Liu, Jie]The Institute of Modern Physics, Chinese Academy of Sciences, Gansu Province, Lanzhou; 730000, China
  • [ 13 ] [Guo, Gang]China Institute of Atomic Energy, Beijing; 102413, China
  • [ 14 ] [Shan, Xiaoting]The Key Laboratory of Science and Technology on Silicon Devices, Institute of Microelectronics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 15 ] [Xiong, Guodong]The Key Laboratory of Science and Technology on Silicon Devices, Institute of Microelectronics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 16 ] [Gao, Jiantou]The Key Laboratory of Science and Technology on Silicon Devices, Institute of Microelectronics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 17 ] [He, Chaohui]School of Nuclear Science and Technology, Xi'An JiaoTong University, Shaanxi Province, Xi'an; 710049, China
  • [ 18 ] [Han, Zhengsheng]The University of Chinese Academy of Sciences, Beijing; 100029, China
  • [ 19 ] [Han, Zhengsheng]The Key Laboratory of Science and Technology on Silicon Devices, Institute of Microelectronics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 20 ] [Liu, Xinyu]The University of Chinese Academy of Sciences, Beijing; 100029, China
  • [ 21 ] [Liu, Xinyu]The Key Laboratory of Science and Technology on Silicon Devices, Institute of Microelectronics, Chinese Academy of Sciences, Beijing; 100029, China
  • [ 22 ] [Zhao, Fazhan]The Key Laboratory of Science and Technology on Silicon Devices, Institute of Microelectronics, Chinese Academy of Sciences, Beijing; 100029, China

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Source :

ACS Photonics

Year: 2021

Issue: 10

Volume: 8

Page: 2912-2922

7 . 5 2 9

JCR@2020

ESI Discipline: PHYSICS;

ESI HC Threshold:26

Cited Count:

WoS CC Cited Count: 0

SCOPUS Cited Count: 16

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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