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Abstract:
AlN skeleton structure-reinforced highly oriented graphite flake (AlN/GF) composites have become a promising candidate for thermal management materials owing to their high thermal conductivity and low thermal expansion. However, the applications of AlN/GF composites are still limited by their poor mechanical properties. Herein, a carbon nanotube-coated alumina (Al2O3@CNT) hybrid was used as a reinforcement to improve the mechanical performance of AlN/GF composites prepared via vacuum infiltration followed by spark plasma sintering. It was found that the relative density and orientation degree of the composites decreased slightly with an increase in the Al2O3@CNT content from 0 to 2 wt%. However, the fracture toughness and bending strength of the composites improved significantly after the introduction of the Al2O3@CNT hybrid reaching up to 1.66 MPam1/2 and 95 MPa, respectively, which correspond to an improvement of approximately 50% and 20% over those of the AlN/GF composite. With the addition of the Al2O3@CNTs, the thermal expansion of the composites increased from 7.3 × 10-6/K to ∼15.5 × 10-6/K, while the thermal conductivity decreased from 442 to ∼253 W/m/K. The toughening and strengthening mechanisms as well as the thermal impact mechanism of the composites were also investigated. © 2021 Elsevier Ltd and Techna Group S.r.l.
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Ceramics International
ISSN: 0272-8842
Year: 2021
Issue: 3
Volume: 48
Page: 4276-4284
4 . 5 2 7
JCR@2020
ESI Discipline: MATERIALS SCIENCE;
ESI HC Threshold:36
Cited Count:
SCOPUS Cited Count: 2
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 11
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