The　growing　demand　for　storage　space　has　promoted　in-depth　research　on　magnetic　performance　regulation　in　an　energysaving　way.　Recently,　we　developed　a　solar　control　of　magnetism,　allowing　the　magnetic　moment　to　be　manipulated　by　sunlight　instead　of　the　magnetic　field,　current,　or　laser.　Here,　binary　and　ternary　photoactive　systems　with　different　photon-to-electron　conversions　are　proposed.　The　photovoltaic/magnetic　heterostructures　with　a　ternary　system　induce　larger　magnetic　changes　due　to　higher　short　current　density　(J(SC))　(20.92　mA.cm(-2))　compared　with　the　binary　system　(11.94　mA.cm(-2)).　During　the　sunlight　illumination,　ferromagnetic　resonance　(FMR)　shift　increases　by　80%　(from　169.52　to　305.48　Oe)　attributed　to　enhanced　photoinduced　electrons　doping,　and　the　variation　of　saturation　magnetization　(M-S)　is　also　amplified　by　14%　(from　9.9%　to　11.3%).　Furthermore,　photovoltaic　performance　analysis　and　the　transient　absorption　(TA)　spectra　indicate　that　the　current　density　plays　a　major　role　in　visible　light　manipulating　magnetism.　These　findings　clarify　the　laws　of　sunlight　control　of　magnetism　and　lay　the　foundation　for　the　next　generation　solar-driven　magneto-optical　memory　applications.